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Inthiswork,weaimatdevelopingtheclickreactionintoausefulpolymerizationtechnique.Whereasthermal1,4-dipolarpolycycloadditionisregiorandom,wesucceededinthedevelopmentofthermallyactivated,metal-free,regioselectiveclickpolymerizations.Usingcopperandruthenium-mediatedclickpolymerizations,wesuccessfullysynthesizedsoluble,1,4-and1,5-regioregularpolytriazoleswithlinearandhyperbranchedstructures. |
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